I've been adjusting the rangefinder alignment on my 4x5 Linhof Technika V, and made some pictures to help me remember the procedure for next time.
Before starting, make sure the lens is pulled out to the infinity stops, and that infinity is focused properly on the ground glass. Next ensure that the back is fully in contact with the body and the rear back adustment knobs are locked. Make sure the cam is the correct one for the lens. Make sure the front focus tracks are in the normal infinity position. Once all that is done and checked, the rangefinder image should be properly lined up when looking at an object a few hundred yards or more away. If not, then the rangefinder needs to be adjusted.
The rangefinder can be adjusted both vertically and horizontally. The vertical image alignment changes as you focus, so you want the focus position to be at infinity for adjustment. The vertical adjustment screw is down at the bottom of the rangefinder housing (see photos 1 and 2). You'll have to peel back some of the leather covering, and remove a thin metal cover plate over the access hole. Sometimes the thin metal cover plate is missing, or might come off when you peel back the leather covering. Try not to lose it, but it's probably not the end of the world if you do. The screw has a blade type end, but the slot is a bit thin for most standard screwdrivers. Get a quality precision screwdriver that fits properly, since you don't want to damage the slot.
To adjust the vertical alignment at infinity, you'll need to be outside so you can view a very distant object (few hundred yards at least) through the rangefinder. This obviously needs to be done with a camera on a firm tripod. Choose a day with little or no wind, and bright conditions. The rangefinder has both a fixed and moving image that need to be aligned at infinity. If they're not aligned, determine if the moving image is above or below the fixed image. To do that, change the focus thumbwheel to determine which is the moving image, and focus back to infinity. The moving image goes down when you tighten the vertical alignment screw (clockwise). The moving image goes up when you loosen the vertical alignment screw. Once you've got alignment at infinity you put back the thin metal cover and leather with a bit of contact cement.
The horizontal alignment is done with a screw that's accessed from a small hole just above the flash mounting bracket (see photos 3 and 4). To gain access, remove the flash mounting bracket via the two screws. Next remove some of the leather covering (and thin metal plate if there). The screw is quite deep in the housing, and the hole is relatively small, so it's difficult to see once you try to get a precision screwdriver in there. For easier viewing, it should be possible to unscrew the rear rangefinder eyepiece to allow some light in from there. I don't remember which screw tightening direction moves the image left or right, so you'll have to try it out each way.
These instructions are for the 4x5 Technika V, and i'm pretty sure they're similiar for the IV and Master. The Technika III seems to be different, and I've never owned one, so don't assume this will work.
I should also add that if you're using cams for more than one lens, you should check the infinity position with all your lenses before making any rangefinder adjustments. If the rangefinder vertical alignment is out in the same way for all your lenses/cams, then the rangefinder is out of alignment and needs to be adjusted. On the other hand, if the vertical alignment is only bad for one lens/cam, then the problem may be with that cam rather than the rangefinder. Keep in mind that changing the rangefinder infinity alignment will affect all your cams, not just the one you're adjusting. Mismatched cams and lenses is not unusual, especially if you're buying used, so I wouldn't expect you could adjust for multiple cams/lenses unless they were all matched and cut by Linhof.
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