Unsharp Masking, Smart Sharpen, Hi-Pass sharpening*, and of course Layers/Masks make Photoshop a much more powerful tool than Lightroom. If you want to optimize for really large prints, do it in PS and forget about LR. It's a pain bouncing around programs anyway IMO, especially with large files.
*This is a technique, not a sharpening algorithm. Google it and learn the technique, and then you can make a simple Photoshop Action to perform it quickly. This type of sharpening is very powerful.
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